This study explores the benefits of a triple-layer remote phosphor structure for white light-emitting diodes (WLEDs) to enhance angular color uniformity and luminous efficiency. Compared to dual-layer structures, the triple-layer configuration showed superior color quality scales (CQS) and luminous flux at various correlated color temperatures. Experimental results indicate that the triple-layer design, incorporating green and red phosphors, improves both color uniformity and luminous efficiency, providing valuable insights for WLED manufacturers.